Anhui Provincial Key Laboratory of Advanced Functional Materials and Devices

Hefei, China

Anhui Provincial Key Laboratory of Advanced Functional Materials and Devices

Hefei, China
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Liu J.-Q.,Hefei University of Technology | Liu J.-Q.,Anhui Provincial Key Laboratory of Advanced Functional Materials and Devices | Liu J.-Q.,Australian National University | Dai M.-J.,Hefei University of Technology | And 5 more authors.
Optoelectronics Letters | Year: 2017

Unique multiple heterojunction of Pt-BiOBr/TiO2 nanotube arrays (Pt-BiOBr/TNTAs) was achived by successively loading both Pt nanoparticles (NPs) and BiOBr nanoflkes (NFs) on surface of ordered and spaced TiO2 nanotubes (NTs) using anodization followed by solvothermal and sequential chemical bath deposition (S-CBD) method. The fabricated Pt-BiOBr/TNTAs were fully characterized, and the photocatalytic (PC) activity and stability of Pt-BiOBr/TNTAs toward degradation of methyl orange (MO) under visible-light irradiation (λ>400 nm) were evaluated. The results reveal that multiple heterostructures of Pt/TiO2, Pt/BiOBr and BiOBr/TiO2 are constructed among TNTAs substrate, Pt NPs and BiOBr NFs, and the hybrid Pt-BiOBr/TNTAs catalyst exhibits remarkable visible-light PC activity, favourable reusability and long-term stability. The combined effect of several factors may contribute to the remarkable PC performance, including strong visible-light absorption by both Pt NPs and BiOBr NFs, lower recombination rate of photo-generated electrons and holes attributed to the multiple heterojunction, microstructures for facile light injection and adsorption as well as efficient mass transport, and larger specific surface area for enhancing light absorption, increasing the effective contact area between the absorbed dye molecules and catalyst and benefiting the molecule transport of reactants or products. © 2017, Tianjin University of Technology and Springer-Verlag Berlin Heidelberg.


Liu L.,Hefei University of Technology | Liu L.,Anhui Provincial Key Laboratory of Advanced Functional Materials and Devices | Hui J.,Hefei University of Technology | Hui J.,Anhui Provincial Key Laboratory of Advanced Functional Materials and Devices | And 7 more authors.
Materials Letters | Year: 2014

Highly detached TiO2 nanotube arrays (TiO2-NTAs) were fabricated by anodization method using electrolyte with high water content. CdS and CdSe quantum dots (QDs) were co-deposited on the TiO2-NTAs. The results showed that the CdS and CdSe QDs were uniformly deposited on both the outer wall and inner tube of TiO2-NTAs. The photocatalytic performance of the as-prepared (CdS-CdSe)/TiO2-NTAs was tested by degradation of methyl orange with 0.2 M Na2S and Na 2SO3 as sacrificial reagents under visible light (λ>400 nm). It was found that the photodegradation rate reached as high as 95.1% in 2 h. Also, a reasonable degradation rate of 87.5% was achieved after 3 cycles, suggesting a good stability of the as-prepared (CdS-CdSe)/TiO2-NTAs. © 2014 Elsevier B.V.


Liu L.,Hefei University of Technology | Liu L.,Anhui Provincial Key Laboratory of Advanced Functional Materials and Devices | Lv J.,Hefei University of Technology | Lv J.,Anhui Provincial Key Laboratory of Advanced Functional Materials and Devices | And 9 more authors.
Journal of Solid State Chemistry | Year: 2013

In this study, TiO2 nanotube arrays (TiO2-NTs) with various intertube spaces were fabricated in the electrolyte with different water contents and the CdS nanoparticles (CdS NPs) were further deposited onto the TiO2-NTs as a sensitizer via a sequential chemical bath deposition (S-CBD) method. The FE-SEM, TEM, XRD and XPS results demonstrated that the CdS NPs were uniformly deposited onto the surface of TiO2-NTs. It was found that higher water content in electrolyte was in favor of large intertube space and pore size and the uniform deposition of CdS NPs. The photocatalytic degradation of methyl orange was tested with the as-prepared CdS/TiO 2-NTs under visible light (λ>400 nm). It was found that the photodegradation rate reached as high as 96.7% under visible irradiation for 180 min. In addition, a reasonable degradation rate of 75.8% was achieved even after 5 cycles, suggesting a good photocatalytic stability of the as-prepared CdS/TiO2-NTs. © 2013 Elsevier Inc.

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